A Simple and Efficient Process for Large Scale Glycerol Oligomerization by Microwave Irradiation

نویسندگان

  • Rémi Nguyen
  • Nicolas Galy
  • Abhishek K. Singh
  • Florian Paulus
  • Daniel Stöbener
  • Cathleen Schlesener
  • Sunil K. Sharma
  • Rainer Haag
چکیده

Herein, an optimized method for 100 g scale synthesis of glycerol oligomers using a microwave multimode source and the low priced K2CO3 as catalyst is reported. This method allows the complete conversion of glycerol to its oligomers in only 30 min, yielding molecular weights up to 1000 g mol−1. Furthermore, a simple iterative purification process, involving the precipitation of the crude product in acetone and methanol, affords a final product composed of larger oligomers with a narrow dispersity (D < 1.5).

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

A Tandem Scalable Microwave-Assisted Williamson Alkyl Aryl Ether Synthesis under Mild Conditions

An efficient tandem synthesis of alkyl aryl ethers, including valuable building blocks of dialdehyde and dinitro groups under microwave irradiation and solvent free conditions on potassium carbonate as a mild solid base has been developed. A series of alkyl aryl ethers were obtained from alcohols in excellent yields by following the Williamson ether synthesis protocol under practical mild condi...

متن کامل

Microwave-assisted Decomposition of two Simple Zinc(II) Schiff Base Complexes: A Facile and Fast Route to Synthesize ZnO Nanostructures

ZnO nanorods and nanoparticles have been easily prepared via the decomposition of two simple Schiff base zinc (II) complexes, namely (N,N'–disalicylalethylenediamine)zince(II) and (N,N'–disalicylalphenylenediamine)zince(II) under microwave irradiation. The decomposition products of the complexes were characterized by FT-IR, XRD, SEM, EDX and UV-visible spectroscopy.  FT-IR, XRD and EDX results ...

متن کامل

ZrP2O7 nanoparticles as a robust and efficient catalyst for the synthesis of 2-aryl-5-methyl-2,3-dihydro-1H-3-pyrazolones under microwave irradiation

ZrP2O7 nanoparticles have been used as an efficient catalyst for the preparation of 2-aryl-5-methyl-2,3-dihydro-1H-3-pyrazolones by a simple one-pot four-component reaction of phenyl hydrazines, ethyl acetoacetate ,β-naphthol and benzaldehydes under microwave irradiation in good to excellent yields. When the reaction was carried out using ZrOCl2.8H2O, ZrO2 and ZrP2O7 NPs as the catalyst, the pr...

متن کامل

H3PW12O40 as an efficient catalyst for one-pot- tricomponent synthesis of chromeno[4,3-b]quinolones under microwave irradiation

Some Chromeno[4,3-b]quinoline derivatives were synthesized in a tricomponents one-pot reaction of 1,3-cyclohexadione arylaldehydes and 4-aminocoumarin under Microwave irradiation in the solventless system by using a heteropolyacid catalyst ,H3[PW12O40] in 80-95% yields and high rates. The shorter reaction times, one-pot, good yields, simple work-up procedure and environmentally friendly conditi...

متن کامل

Isolation of borneol and bornyl acetate from Ferulago macrocarpa by microwave irradiation

Background & Aim: A simple and rapid microwave- assisted extraction (MAE) procedure was developed and optimized for the isolation of borneol and bornyl acetate from Ferulago macrocarpa. Ferulago macrocarpa (Apiaceae) is an endemic plant in Iran. Experimental: Dried powdered aerial parts of plants were soaked in water and irradiated with microwave in a Clevenger extraction app...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 2017